He called on Iran to provide access to the Parchin military complex, where the Islamic Republic is believed to have tested rockets.
CNN: Story highlights
He also called on Iran to cooperate with IAEA inspectors over its nuclear program, which Tehran insists is intended solely for peaceful purposes.
CNN: Iran: Ready to work with Obama
In February, Mr Jalili wrote back that Iran was ready for dialogue on what he called a spectrum of issues.
BBC: Fresh Iran nuclear talks agreed with world powers - EU
He has called on western powers to tone down their bellicose rhetoric and in the past has suggested that Iran should be allowed to enrich small amounts of uranium.
ECONOMIST: Iran's president visits New York
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